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Activated Aging Dynamics and Negative Fluctuation-Dissipation Ratios

Peter Mayer, Sébastien Léonard, Ludovic Berthier, Juan P. Garrahan, and Peter Sollich
Phys. Rev. Lett. 96, 030602 – Published 25 January 2006

Abstract

In glassy materials, aging proceeds at large times via thermal activation. We show that this can lead to negative dynamical response functions and novel and well-defined violations of the fluctuation-dissipation theorem, in particular, negative fluctuation-dissipation ratios. Our analysis is based on detailed theoretical and numerical results for the activated aging regime of simple kinetically constrained models. The results are relevant to a variety of physical situations, such as aging in glass formers, thermally activated domain growth, and granular compaction.

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  • Received 29 August 2005

DOI:https://doi.org/10.1103/PhysRevLett.96.030602

©2006 American Physical Society

Authors & Affiliations

Peter Mayer1,2, Sébastien Léonard3, Ludovic Berthier3, Juan P. Garrahan4, and Peter Sollich2

  • 1Department of Chemistry, Columbia University, 3000 Broadway, New York, New York 10027, USA
  • 2Department of Mathematics, King’s College London, London WC2R 2LS, United Kingdom
  • 3Laboratoire des Colloïdes, Verres et Nanomatériaux UMR 5587, Université Montpellier II and CNRS, 34095 Montpellier Cedex 5, France
  • 4School of Physics and Astronomy, University of Nottingham, Nottingham NG7 2RD, United Kingdom

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Issue

Vol. 96, Iss. 3 — 27 January 2006

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